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Accounts of Chemical Research

Subject Areas: Chemistry (miscellaneous)
Publisher: American Chemical Society - American Chemical Society
ISSN: 1520-4898
SJR: 415

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Journal Article

Single-Molecule Correlated Chemical Probing: A Revolution in RNA Structure Analysis

Mustoe, Anthony M.; Weidmann, Chase A.; Weeks, Kevin M.

2023 Accounts of Chemical Research

doi:10.1021/acs.accounts.2c00782 pmid:36917683

Conspectus RNA molecules convey biological information both in their linear sequence and in their base-paired secondary and tertiary structures. Chemical probing experiments, which involve treating an RNA with a reagent that modifies conformationally dynamic nucleotides, have broadly enabled...
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Journal Article

Toward Understanding the Subcellular Distributions of Cholesterol and Sphingolipids Using High-Resolution NanoSIMS Imaging

Brunet, Melanie A.; Kraft, Mary L.

2023 Accounts of Chemical Research

doi:10.1021/acs.accounts.2c00760 pmid:36913670

Conspectus Characterizing the subcellular distributions of biomolecules of interest is a basic inquiry that helps inform on the potential roles of these molecules in biological functions. Presently, the functions of specific lipid species and cholesterol are not well understood, partially...
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Journal Article

Urea- and Thiourea-Based Receptors for Anion Binding

Kundu, Sanchita; Egboluche, Tochukwu Kevin; Hossain, Md. Alamgir

2023 Accounts of Chemical Research

doi:10.1021/acs.accounts.2c00701

Conspectus Over the past five decades, significant progress has been made in the field of anion recognition with a diverse variety of synthetic receptors because of the fundamental importance of anions in chemical, environmental, and biological processes. In particular, urea- and thiourea-based...
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Journal Article

Design, Synthesis, and Evaluation of Allosteric Effectors for Hemoglobin

Enakaya, Nyesa A.; Jefferson, Aniah; Chew-Martinez, Danielle; Matthews, Jason S.

2023 Accounts of Chemical Research

doi:10.1021/acs.accounts.2c00590 pmid:36946781

Conspectus Sickle cell disease (SCD) is an inherited blood disorder caused by a point mutation in hemoglobin (Hb), the protein in the red blood cell (RBC) responsible for the transport of oxygen (O2) throughout the body. The mutation leads to the expression of sickle cell hemoglobin (HbS). Both...
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Journal Article

Predicting Kinetics and Dynamics of Spin-Dependent Processes

Dergachev, Ilya D.; Dergachev, Vsevolod D.; Rooein, Mitra; Mirzanejad, Amir; Varganov, Sergey A.

2023 Accounts of Chemical Research

doi:10.1021/acs.accounts.2c00843

Conspectus Predicting mechanisms and rates of nonadiabatic spin-dependent processes including photoinduced intersystem crossings, thermally activated spin-forbidden reactions, and spin crossovers in metal centers is a very active field of research. These processes play critical roles in...
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Journal Article

Determinants of SuperselectivityPractical Concepts for Application in Biology and Medicine

Dubacheva, Galina V.; Curk, Tine; Richter, Ralf P.

2023 Accounts of Chemical Research

doi:10.1021/acs.accounts.2c00672 pmid:36916901

Conspectus Multivalent interactions are common in biological systems and are also widely deployed for targeting applications in biomedicine. A unique feature of multivalent binding is “superselectivity”. Superselectivity refers to the sharp discrimination of surfaces (e.g., on cells or cell...
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Journal Article

Through the Looking Glass: Using the Lens of [SNS]-Pincer Ligands to Examine First-Row Metal Bifunctional Catalysts

Elsby, Matthew R.; Baker, R. Tom

2023 Accounts of Chemical Research

doi:10.1021/acs.accounts.2c00798 pmid:36921212

Conspectus Homogeneous catalysis is at the forefront of global efforts to innovate the synthesis of fine chemicals and achieve carbon-neutrality in energy applications. For decades, the push toward sustainable catalysis has focused on the development of first-row transition metal catalysts to...
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Journal Article

Understanding and Expanding the Prospects for Electrosynthesis with Liquid Metal Electrodes

Wu, Henry; Hazelnis, Joshua P.; Maldonado, Stephen

2023 Accounts of Chemical Research

doi:10.1021/acs.accounts.2c00850 pmid:36921297

Conspectus This Account describes and summarizes the latest work from our laboratory on developing and maturing strategies based on low-temperature liquid metals as reaction environments for materials synthesis. The electrochemical liquid–liquid–solid (ec-LLS) crystal growth concept is a hybrid...
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Journal Article

Recognition-Encoded Synthetic Information Molecules

Iadevaia, Giulia; Hunter, Christopher A.

2023 Accounts of Chemical Research

doi:10.1021/acs.accounts.3c00029 pmid:36894535

Conspectus Nucleic acids represent a unique class of highly programmable molecules, where the sequence of monomer units incorporated into the polymer chain can be read through duplex formation with a complementary oligomer. It should be possible to encode information in synthetic oligomers as a...
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Journal Article

Selective Control and Characteristics of Water Oxidation and Dioxygen Reduction in Environmental Photo(electro)catalytic Systems

Lee, Shinbi; Bae, Ho-Sub; Choi, Wonyong

2023 Accounts of Chemical Research

doi:10.1021/acs.accounts.3c00002 pmid:36947463

Conspectus Employing semiconductor materials is a popular engineering method to harvest solar energy, which is widely investigated for photocatalysis (PC) and photoelectrocatalysis (PEC) that convert solar light to chemical energy. In particular, environmental photo(electro)catalysis has been...

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