Reactive Bubbly FlowsInvestigation of the Influence of Transport Processes on Chemical Reactions in Bubbly Flows Using Space-Resolved In Situ Analytics and Simultaneous Characterization of Bubble Dynamics in Real-Time
Reactive Bubbly Flows: Investigation of the Influence of Transport Processes on Chemical...
Guhathakurta, Jajnabalkya; Schurr, Daniela; Rinke, Günter; Grottke, Daniel; Kraut, Manfred; Dittmeyer, Roland; Simon, Sven
2021-07-30 00:00:00
[For investigations of concentration profiles around bubbles in millichannels as Taylor flow and in bubble columns two in situ real-time process analysis systems were developed. The first system uses laser Raman spectroscopy combined with real-time digital holography. The Raman part of the system is based on a custom pulsed high-energy laser. With this process analysis system, it is possible to measure concentrations of many chemical compounds selectively, with a spatial resolution in the micrometer range during a 10 µs laser pulse. Due to the two combined principles, the determination of the position of a measured local concentration relative to the gas bubble is possible and has been demonstrated. The second real-time process analysis system is especially suited for colored chemical reactions. The system is based on real-time UV/VIS 2D tomography such that with time the third dimension of a 3D concentration profile in the bubble wake can be determined. It consists of fast line sensors illuminated by a laser light sheet. This light sheet originates from a laser spot moving around one third of the bubble column repeatedly. This system is applicable to freely ascending single bubbles as well as bubbly flows in bubble columns.]
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Reactive Bubbly FlowsInvestigation of the Influence of Transport Processes on Chemical Reactions in Bubbly Flows Using Space-Resolved In Situ Analytics and Simultaneous Characterization of Bubble Dynamics in Real-Time
[For investigations of concentration profiles around bubbles in millichannels as Taylor flow and in bubble columns two in situ real-time process analysis systems were developed. The first system uses laser Raman spectroscopy combined with real-time digital holography. The Raman part of the system is based on a custom pulsed high-energy laser. With this process analysis system, it is possible to measure concentrations of many chemical compounds selectively, with a spatial resolution in the micrometer range during a 10 µs laser pulse. Due to the two combined principles, the determination of the position of a measured local concentration relative to the gas bubble is possible and has been demonstrated. The second real-time process analysis system is especially suited for colored chemical reactions. The system is based on real-time UV/VIS 2D tomography such that with time the third dimension of a 3D concentration profile in the bubble wake can be determined. It consists of fast line sensors illuminated by a laser light sheet. This light sheet originates from a laser spot moving around one third of the bubble column repeatedly. This system is applicable to freely ascending single bubbles as well as bubbly flows in bubble columns.]
Published: Jul 30, 2021
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