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Numerical Analysis and Optimization of a Hybrid Layer Structure for Triplet–Triplet Fusion Mechanism in Organic Light‐Emitting Diodes

Numerical Analysis and Optimization of a Hybrid Layer Structure for Triplet–Triplet Fusion... In this study, a steady state and time‐dependent exciton diffusion model including singlet and triplet excitons coupled with a modified Poisson and drift‐diffusion solver to explain the mechanism of hyper triplet–triplet fusion (TTF) organic light‐emitting diodes (OLEDs) is developed. Using this modified simulator, various characteristics of OLEDs, including the current‐voltage curve, internal quantum efficiency, transient spectrum, and electric profile are demonstrated. This solver can also be used to explain the mechanism of hyper‐TTF‐OLEDs and analyze the loss from different exciton mechanisms. Furthermore, we perform additional optimization of hyper‐TTF‐OLEDs that increases the internal quantum efficiency by ≈33% (from 29% to 40%). http://www.deepdyve.com/assets/images/DeepDyve-Logo-lg.png Advanced Theory and Simulations Wiley

Numerical Analysis and Optimization of a Hybrid Layer Structure for Triplet–Triplet Fusion Mechanism in Organic Light‐Emitting Diodes

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Publisher
Wiley
Copyright
© 2023 Wiley‐VCH GmbH
eISSN
2513-0390
DOI
10.1002/adts.202200633
Publisher site
See Article on Publisher Site

Abstract

In this study, a steady state and time‐dependent exciton diffusion model including singlet and triplet excitons coupled with a modified Poisson and drift‐diffusion solver to explain the mechanism of hyper triplet–triplet fusion (TTF) organic light‐emitting diodes (OLEDs) is developed. Using this modified simulator, various characteristics of OLEDs, including the current‐voltage curve, internal quantum efficiency, transient spectrum, and electric profile are demonstrated. This solver can also be used to explain the mechanism of hyper‐TTF‐OLEDs and analyze the loss from different exciton mechanisms. Furthermore, we perform additional optimization of hyper‐TTF‐OLEDs that increases the internal quantum efficiency by ≈33% (from 29% to 40%).

Journal

Advanced Theory and SimulationsWiley

Published: Feb 1, 2023

Keywords: device modeling; organic light‐emitting diodes; triplet– triplet fusion

References